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No, Chart is effectively `helm template`
You'd need to use the `Release` resource.

Worth reading this: <https://www.pulumi.com/registry/packages/kubernetes/how-to-guides/choosing-the-right-helm-resource-for-your-use-case/|https://www.pulumi.com/registry/packages/kubernetes/how-to-guides/choosing-the-right-helm-resource-for-your-use-case/>

Also worth opening an issue to have the page give clarity on things like `lookup`