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I wasn't making the Values map of maps correctly:
```                _, err = helm.NewChart(ctx, "influx", helm.ChartArgs{
                        Repo: pulumi.String("influxdata"),
                        Chart: pulumi.String("influxdb2"),
                        Values: pulumi.Map{
                                "persistence": pulumi.Map{
                                        "storageClass": pulumi.String("efs-stor"),
                                        "size": pulumi.String("52Gi"),
                                },
                        },
                },```
Works.

Sorry for the SPAM