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I think this is what the <https://www.pulumi.com/registry/packages/kubernetes/api-docs/helm/v3/release/#values_csharp|Values> property is for.

Yes. I tried populating the values dictionary but it has no effect when referencing a local chart.

Just to follow up. I discovered that if your local chart has a `values.yaml` defined it will ignore any values passed in via the `Values` parameter. If you want to mix code and yaml defined variables you need to keep the yaml external to the local chart.