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Is there a mechanism to modify an object after it has been initialized but before the Language Host program exits? In my case I am trying to set the ResourceOptions.import setting on an s3.Bucket that is nested within a couple layers of ComponentResource.

Not yet - but we're actively working on it now at <https://github.com/pulumi/pulumi/issues/2068> (and <https://github.com/pulumi/pulumi/pull/3174>).